Structural characterisation of chemisorbed methoxy in ZSM5: an intermediate in the methanol-to-gasoline process

DOI

Zeolites and zeotype materials are well established in the field of catalytic science. Particularly notable is their use for shape selective, acid-catalyzed conversions of simple hydrocarbons to alcohols, alkenes and aromatics. H-ZSM5 is a well-established catalyst for the commercially important methanol-to-gasoline and methanol-to-olefin processes. For both of these, the first step is to activate methanol by chemisorbing it to the zeolite to generate a chemisorbed methoxy species. The aim of this proposal is to structurally characterise the chemisorbed methoxy group using total scattering neutron diffraction. This will be the first time a reaction intermediate has been structurally characterised inside a zeolite.

Identifier
DOI https://doi.org/10.5286/ISIS.E.67772945
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/67772945
Provenance
Creator Professor Richard Catlow; Dr Ian Silverwood; Professor Stewart Parker; Dr Alexander O'Malley; Dr Sam Callear; Dr Arun Chutia
Publisher ISIS Neutron and Muon Source
Publication Year 2018
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2015-12-14T09:00:00Z
Temporal Coverage End 2015-12-17T09:00:00Z