Observation of a new degradation mechanism involving electrocatalyst nanoparticle growth in hydrogen PEM fuel cells associated to reduction

DOI

We aim to elucidate the relationship between oxidation state and stability of electrocatalyst for automotive proton exchange membrane fuel cells (PEMFCs) by operando and in situ characterization. The structural evolution of Pt nanoparticles will be tracked in a representative device under accelerated protocols able to capture the effect of low potential excursions, which occur in the application during the stops and were recently recognized as critical for Pt nanoparticles growth and dissolution. The mechanisms (oxidation/reduction, morphological reconstruction, dissolution) rising under the cathodic scan to low potential (<0.4 V) will be elucidated by W/SAXS techniques. The study of different catalyst coated membranes and operating PEMFC conditions can clarify the electrochemical drivers that lead the degradation in this process. The work helps to improve aging mitigation strategies and Pt degradation model, and define PEMFC operational boundaries in dependence on material properties.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-1550921429
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/1550921429
Provenance
Creator Meryem ENNAJI; Raphael CHATTOT (ORCID: 0000-0001-6169-530X); Andrea BARICCI ORCID logo; Laure GUETAZ ORCID logo; Andrea CASALEGNO; Elena COLOMBO ORCID logo; Pol SALLÉS PERRAMON (ORCID: 0000-0003-1426-611X); David MARECEK
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2027
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields