Investigation of hydrogen dynamics on pure and metal cluster decorated metal oxides

DOI

Metal oxides(MO) are widely used in technological applications especially for catalysts and supports for catalysts. We propose to use the inelastic response of H2 adsorbed on well-characterized pure and metal (Pd, Au) decorated ZnO and MgO nanoparticles to probe the molecule metal and molecule MO interactions in a prototype study of catalysts that are used in the production of fine chemicals like H2O2. This proposal is the next phase of our study of the surface mediated chemical reactivity of pure and doped MO nanomaterials. We will extend and enhance the knowledge gained from our earlier published work on H2 dynamics on MgO, ZnO and Graphite to advance the current knowledge base of these important systems. We will combine Z contrast <1Å resolution STEM, state of the art ab initio DFT, thermodynamics and reaction kinetics, TGA and UV -VIS to complement this INS study.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24079499
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24079499
Provenance
Creator Dr Anibal Ramirez-Cuesta; Dr John Larese; Ms Paige Landry; Dr Thomas Arnold; Mr Andy Hicks
Publisher ISIS Neutron and Muon Source
Publication Year 2013
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2010-07-09T08:25:47Z
Temporal Coverage End 2010-07-16T10:11:56Z