Simultaneous microwave dielectric spectroscopy and neutron diffraction of Transition Metal Halides Ammoniates (Cu[NH3]nX2

DOI

We have constructed a novel microwave frequency resonator that can sit within the GEM and POLARIS diffractometers and will allow us to simultaneously collect diffraction and dielectric data for sample materials. We request beam time on POLARIS or GEM to collect simultaneous structural, dielectric and mass spectroscopy data on a new series of compounds, the ammoniates of the cupric halides, CuCl2, CuBr2 and CuI2. The structures of these materials are well know1, 2 in both the diammine, Cu[NH3]2X2, and hexa-ammine, Cu[NH3]6X2, forms. These compounds show good thermal stability, with the diammoniate (Cu[NH3]2X2) stable beyond 300oC. This high temperature stability is of particular interest for gas-filtering and purification applications where tthe coordinated ammonia can eliminate undesirable components, such as NOx, from exhaust streams without thermal loss of ammonia.

Identifier
DOI https://doi.org/10.5286/ISIS.E.49915730
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/49915730
Provenance
Creator Professor Adrian Porch; Mr Jon Hartley; Dr Martin Jones; Dr Ron Smith
Publisher ISIS Neutron and Muon Source
Publication Year 2017
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2014-06-08T23:00:00Z
Temporal Coverage End 2014-06-10T23:00:00Z