Lithium ion distribution in lithium-rich lithium manganese polyphosphate electrode glasses for lithium batteries

DOI

The present proposal seeks to establish the conductivity mechanism in a series of lithium manganese polyphosphate glasses rich in lithium for potential use in all solid state lithium ion batteries. Lithium ion distribution and the role of manganese will be investigated by a combination of neutron and X-ray scattering data analysis. Data will be analysed to reveal short range correlations and average coordination numbers. Key to establishing the conductivity mechanism is direct investigation of the Li-Li correlations. These will be examined by appropriate subtraction of data obtained from null-Li containing. Energy minimised structural models will be constructed for use as starting models for Reverse Monte Carlo fitting of the real space and reciprocal space data to reveal detail of the longer range correlations.

Identifier
DOI https://doi.org/10.5286/ISIS.E.58448711
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/58448711
Provenance
Creator Mr Ali Shehu; Mr Lei Wang; Dr Alex Hannon; Dr Isaac Abrahams; Professor Martin Dove
Publisher ISIS Neutron and Muon Source
Publication Year 2018
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2015-04-13T08:00:00Z
Temporal Coverage End 2015-06-22T15:27:53Z