In this proposal we wish to explore how the RF-MuSR technique might be developed for measurements akin to FT-NMR. Our work will focus on the broadband excitation of paramagnetic systems where a short, intense RF pulse excites a band of frequencies centred on the RF carrier that are measured simultaneously in the free precession signal. This continuation proposal will focus on the application of the technique to the measurement of free precession signals for muoniated radicals, using norbornene as a test system.