Crystallization of clathrate hydrates from amorphous THF-water solutions

DOI

Understanding clathrate hydrate formation and stability is an urgent issue due to their environmental importance. However, a fundamental understanding of the molecular processes governing their formation has remained elusive. We have now developed a novel method of preparing amorphous solutions, which crystallize slowly to cubic structure II clathrate hydrates upon heating in the temperature range 160 - 200 K. In this temperature range we were able to follow by powder X-ray diffraction how one or two unit cells form from the amorphous solution and grow to a crystal of the size of many unit cells. This finding now provides the unique opportunity of studying how the process of clathrate nucleation and growth takes place on the molecular level. This requires study of a set of isotopically substituted amorphous solutions and extraction of partials from neutron data.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24079586
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24079586
Provenance
Creator Professor John Finney; Dr Daniel Bowron; Dr Katrin Winkel; Professor Thomas Loerting; Dr Marion Bauer
Publisher ISIS Neutron and Muon Source
Publication Year 2013
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2010-07-19T08:50:01Z
Temporal Coverage End 2010-07-24T07:46:15Z