Separation of factors contributing to the overall diffusion behaviour of olefin species in catalytic zeotype structures.

DOI

This proposal examines the diffusion behaviour of olefin hydrocarbons adsorbed in microporous zeolite catalysts. It builds on a previous study which has shown that simulated aging of the catalyst results in changes to the diffusion behaviour of the adsorbed species and seeks to distinguish how each aspect of the aging-related alterations to the zeolite contribute to the overall change in olefin diffusion. These differences in diffusion are a key factor in determining the selectivity of the catalyst toward different reaction pathways, which makes important contributions to its commercial application in both catalytic cracking and methanol-to-gasoline processes.

Identifier
DOI https://doi.org/10.5286/ISIS.E.RB1920592-1
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/108665575
Provenance
Creator Dr Ian Silverwood; Professor Russell Howe; Dr Alexander Hawkins; Professor David Lennon; Dr Iain Hitchcock; Ms Andrea Zachariou
Publisher ISIS Neutron and Muon Source
Publication Year 2022
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2019-11-14T09:04:16Z
Temporal Coverage End 2019-11-20T09:35:06Z