Null Isotope Study of Lithium Borogermanate Glasses - continuation

DOI

Alkali borogermanate glasses are topologically complex, in that [BOn] (n = 3, 4)and [GeOn] (n = 4, 5, 6) polyhedra can coexist. Equilibrium between these structural units has significant influence on physico-chemical properties such as conductivity and corrosion resistance. In previous work on the potassium system we used neutron diffraction and NMR to show that K preferentially associates with borate units to form [BO4] in preference to [GeO5,6], giving an increase in average coordination of B from 3 to 3.8 but of Ge from 4 to only 4.3. We have repeated the study with the lithium system taking advantage of the opposite signs of the scattering lengths of the Li-6 and Li-7 isotopes to produce samples which show null scattering from Li. The data then showed contributions only from the [BOn] and [GeOn] polyhedra. We now need data from natural Li isotope samples to study the Li environment.

Identifier
DOI https://doi.org/10.5286/ISIS.E.83552832
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/83552832
Provenance
Creator Dr Alex Hannon; Dr Oliver Alderman; Dr Diane Holland; Mr Faizani Mohd Noor
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2016-12-05T08:00:00Z
Temporal Coverage End 2016-12-09T08:00:00Z