Light-induced renormalization of the Dirac quasiparticles in the nodal-line semimetal ZrSiSe

In nodal-line semimetals, linearly dispersing states form Dirac loops in the reciprocal space with a high degree of electron-hole symmetry and a reduced density of states near the Fermi level. The result is reduced electronic screening and enhanced correlations between Dirac quasiparticles. Here we investigate the electronic structure of ZrSiSe, by combining time- and angle-resolved photoelectron spectroscopy with ab initio density functional theory (DFT) complemented by an extended Hubbard model (DFT+U+V) and by time-dependent DFT+U+V. We show that electronic correlations are reduced on an ultrashort timescale by optical excitation of high-energy electrons-hole pairs, which transiently screen the Coulomb interaction. Our findings demonstrate an all-optical method for engineering the band structure of a quantum material.

This record contains the ARPES raw data in txt format used to create the figures in the referenced publication.

Identifier
Source https://archive.materialscloud.org/record/2021.122
Metadata Access https://archive.materialscloud.org/xml?verb=GetRecord&metadataPrefix=oai_dc&identifier=oai:materialscloud.org:964
Provenance
Creator Gatti, Gianmarco; Crepaldi, Alberto; Puppin, Michele; Tancogne-Dejean, Nicolas; Xian, Lede; De Giovannini, Umberto; Roth, Silvan; Polishchuk, Serhii; Bugnon, Philippe; Magrez, Arnaud; Berger, Helmuth; Frassetto, Fabio; Poletto, Luca; Moreschini, Luca; Moser, Simon; Bostwick, Aaron; Rotenberg, Eli; Rubio, Angel; Chergui, Majed; Grioni, Marco
Publisher Materials Cloud
Publication Year 2021
Rights info:eu-repo/semantics/openAccess; Creative Commons Attribution 4.0 International https://creativecommons.org/licenses/by/4.0/legalcode
OpenAccess true
Contact archive(at)materialscloud.org
Representation
Language English
Resource Type Dataset
Discipline Materials Science and Engineering