Charge disproportionation and structural modulation in multiferroic CaMn7O12

DOI

Multiferroic materials in which strongly coupled magnetic and ferroelectric order parameters coexist attract considerable interest. Below 90 K, CaMn7O12 possesses the largest magnetically induced polarisation measured to date. With a view to integrate multiferroics in novel technology, understanding the microscopic physics behind this giant polarisation, which has been predicted to be due to exchange-striction between Mn3+ and Mn4+ ions, is of key importance. As described in this proposal, by accurately determining the oxygen positions in CaMn7O12 (impossible with x-ray diffraction techniques) we will be able to determine the potentially critical role of charge disproportionation in creating the electric polarisation. In addition, the collected data would allow a hypothesis of a novel orbital helix method of electronic ordering to be tested, which is thought to occur below 250 K.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24089296
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24089296
Provenance
Creator Professor Paolo Radaelli; Dr Christine Martin; Dr Laurent Chapon; Dr Roger Johnson; Ms Natasha Perks
Publisher ISIS Neutron and Muon Source
Publication Year 2015
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2012-08-02T09:00:06Z
Temporal Coverage End 2012-08-11T12:01:17Z